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- W1748013548 endingPage "200" @default.
- W1748013548 startingPage "192" @default.
- W1748013548 abstract "The fluorinated cyclopentadienyl complexes [Rh(η5-C5H4CH2CH2C6F13)(CO)2] (2), [Rh(η5-C5H4CH2CH2C8F17)(CO)2] (3), [Rh(η5-C5H4CH2CH2C10F21)(CO)2] (4), [Rh(η5-C5H4CH2CH2CnF2n+1)(CO)(PEt3)] (7: n = 6; 8: n = 8; 9: n = 10) and [Rh(η5-C5H4CH2CH2CnF2n+1)(CO){P(CH2CH2C6F13)3}] (10: n = 8; 11: n = 10) were synthesized and their reactivity was investigated. Compound 3 converts at room temperature into the trinuclear complex [Rh2(η5-C5H4CH2CH2C8F17)2(μ-CO)2Rh(η5-C5H4CH2CH2C8F17)(CO)] (6). The complexes 9 and 11 were employed in dehydrogenation reactions of cycloalkanes in C6F14/hydrocarbon mixtures. Photocatalytic conversions were observed and a turnover number of 16 for the dehydrogenation of cyclooctane with complex 11 was obtained." @default.
- W1748013548 created "2016-06-24" @default.
- W1748013548 creator A5035715870 @default.
- W1748013548 creator A5038036379 @default.
- W1748013548 creator A5038277232 @default.
- W1748013548 date "2015-12-01" @default.
- W1748013548 modified "2023-10-17" @default.
- W1748013548 title "Dehydrogenation of cycloalkanes at rhodium complexes bearing fluorinated cyclopentadienyl ligands" @default.
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- W1748013548 doi "https://doi.org/10.1016/j.jfluchem.2015.09.014" @default.
- W1748013548 hasPublicationYear "2015" @default.
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