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- W1776373091 abstract "This chapter discusses magnetic circular dichroism and diamagnetic molecules. Unlike ordinary absorption and natural optical activity, the Faraday effect cannot be evaluated by one or two matrix elements, because the magnetic field provides a static perturbation that mixes all other states with the one being studied. In many instances excited states are classed into groups where it is equally tractable to construct a wave function for one as for another. In this case it may often happen that the greater part of the magnetic circular dichroism (MCD) will come from the mixing of these states. In other cases it will be generally possible to employ an approximate summation or variation technique, particularly at this stage of development where a qualitative understanding of the observed behavior is still to be gained. Among the general factors that appear to play an interesting role in MCD research are vibronic, degeneracy, and spin phenomena. Closely coupled to this behavior is the strength of the transition with the categories, strong, weak, and forbidden often providing qualitatively distinct types. In circular dichroism (CD) spectra weakly allowed transitions give large effects when they are magnetically allowed; however, there are still no well-established reasons for spin-forbidden transitions to play any more important role than they do in ordinary absorption." @default.
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- W1776373091 date "1972-01-01" @default.
- W1776373091 modified "2023-10-06" @default.
- W1776373091 title "Magnetic Circular Dichroism and Diamagnetic Molecules" @default.
- W1776373091 doi "https://doi.org/10.1016/s0065-3276(08)60543-2" @default.
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