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• W1972256961 startingPage "2249" @default.
• W1972256961 abstract "Generation of singlet molecular oxygen ((1)O(2)) by photosensitization with methylene blue (MB) supported in Nafion-Na films has been quantified by integration of the (1)O(2) emission decay at 1270 nm. The quantum yield of (1)O(2) production (Phi(Delta)) in the air-equilibrated solid phase is 0.24 +/- 0.03. Information on the (1)O(2) generation environment has been gained from complementary techniques such as UV-Vis absorption and emission spectroscopy, as well as MB fluorescence and triplet-triplet absorption decay. Results are compared with the (1)O(2) generation by MB in methanol solution (Phi(Delta) = 0.51) and in methanol-swollen Nafion films (Phi(Delta) = 0.49 +/- 0.06). Differences and similarities are discussed in terms of the factors that influence Phi(Delta) in solution and in the solid media. The optical and mechanical features of Nafion, ease of dye loading, compatibility with most solvents, homogeneity, reproducibility and stability of the photosensitizing material makes it a convenient reference for (1)O(2) generation quantum yield measurements in transparent (micro)heterogeneous and homogeneous media." @default.
• W1972256961 created "2016-06-24" @default.
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• W1972256961 date "2006-01-01" @default.
• W1972256961 modified "2023-10-16" @default.
• W1972256961 title "A clean, well-defined solid system for photosensitized¹O₂production measurements" @default.
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• W1972256961 doi "https://doi.org/10.1039/b517756a" @default.
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