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- W1973287872 abstract "Two novel Pb(II)-based metal–organic frameworks (MOFs) based on the rigid bitetrazolate ligand 1,4-benzeneditetrazol-5-yl (H2BDT) have been synthesized under hydrothermal conditions and fully characterized. In these two compounds, [Pb4(OH)4(BDT)2]·2H2O (1) and [Pb4(OH)4(BDT)]·BDT·2H2O (2), the H2BDT ligands exhibit three different coordination modes which are firstly reported in M-BDT frameworks, constructing disparate architectures by bridging the same cubane-shaped [Pb4(OH)4]4+ building units. Compound 1 features a 3D supramolecular network with a rare 2-fold interpenetrating (10, 3)-d (or utp) topology which is accomplished by connecting [Pb4(OH)4]4+ clusters to μ4-bridging BDT2− ligands via weak bonds. Compound 2 exhibits a 2D square grid with (4, 4) topology and the adjacent 2D networks are further linked by Pb–O weak bonds to generate the 3D supramolecular structure. Moreover, the structures of these two compounds are highly influenced by the concentration of the starting reagents. Compounds 1 and 2 exhibit strong solid-state fluorescent emission with millisecond luminescence lifetimes at room temperature." @default.
- W1973287872 created "2016-06-24" @default.
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- W1973287872 date "2012-01-01" @default.
- W1973287872 modified "2023-09-22" @default.
- W1973287872 title "Two novel lead(ii)-tetrazolate frameworks based on cubane [Pb4(OH)4]4+ clusters trapping long lifetime luminescence emission" @default.
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- W1973287872 doi "https://doi.org/10.1039/c2ce25078k" @default.
- W1973287872 hasPublicationYear "2012" @default.
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