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- W1986043826 abstract "Abstract The concept of a transition to an amorphous state as the process of relaxation of a metastable crystalline phase with a higher free energy than the amorphous state is presented. The relaxation is considered as a process of heterogeneous nucleation and growth of amorphous grains in a metastable crystalline matrix. The crystalline phase can be metastable either because of a large defect concentration or because of a non-equilibrium crystalline structure. The assumption of the existence of long-lived crystal-like clusters in a liquid is important for a description of the liquid-glass transition. It is shown that the free energy of a mixture of a gas-like liquid and crystal-like clusters near the melting temperature can be lower than that of a pure gas-like liquid. The quantity of these clusters increases with cooling and the percolation region corresponds to the glass transition interval." @default.
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- W1986043826 date "1990-09-01" @default.
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- W1986043826 title "Phenomenological model of crystal-amorphous phase change" @default.
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- W1986043826 doi "https://doi.org/10.1016/0022-3093(90)91077-5" @default.
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