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• W1993346578 startingPage "281" @default.
• W1993346578 abstract "A phase-modulation technique for coherent Raman spectroscopy is used to measure both the real and imaginary parts of the third-order nonlinear susceptibility of gases. The Raman Q-branch resonance of ${mathrm{D}}_{2}$ is calibrated by comparison to the Q-branch resonance of ${mathrm{N}}_{2}$. By using ${mathrm{D}}_{2}$ as an internal standard, the nonresonant electronic susceptibility of Ar and the sum of the electronic and molecular reorientation contributions to the nonresonant susceptibility of ${mathrm{N}}_{2}$ are determined. The results of these measurements are compared to published data on the Q-branch Raman cross section of ${mathrm{H}}_{2}$, to predictions from the theory of the optical (ac) Kerr effect, and to measurements of electronic hyperpolarizabilities. For the last-mentioned quantity, measurements from three-wave mixing, from field-induced second-harmonic generation, from third-harmonic generation, and from the electro-optic (dc) Kerr effect are intercompared and agreement at the 10% level is established. Formulas interrelating a number of different definitions of third-order susceptibilities found in the literature are presented." @default.
• W1993346578 created "2016-06-24" @default.
• W1993346578 creator A5012926687 @default.
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• W1993346578 date "1985-07-01" @default.
• W1993346578 modified "2023-09-23" @default.
• W1993346578 title "Measurement of resonant and nonresonant third-order nonlinear susceptibilities by coherent Raman spectroscopy" @default.
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• W1993346578 doi "https://doi.org/10.1103/physreva.32.281" @default.
• W1993346578 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/9896052" @default.
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