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• W1997065559 abstract "Infrared spectra of the OCS–He van der Waals complex and of OCS–HeN clusters have been studied in the region of the OCS ν1 fundamental band using a tunable diode laser to probe a pulsed supersonic slit jet. For the complex, the spectrum of the normal isotope, O16C12S32–He4, has been considerably extended and the S34- and C13-substituted forms have been recorded for the first time. The data could be analyzed satisfactorily using a conventional asymmetric rotor Hamiltonian with sextic centrifugal distortion terms. For the clusters, the S34- and C13-substituted forms have been observed and assigned for N=2–7, including some transitions with higher J values than previously reported for the normal isotope, e.g., R(5). The observed vibrational shifts, relative to the free OCS molecule, were very similar to those of the normal isotope, and most of the difference could be explained by simple scaling. These results constitute a subtle and precise probe of intermolecular forces and dynamical effects in a system which is of current interest for cluster studies." @default.
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• W1997065559 date "2006-10-10" @default.
• W1997065559 modified "2023-09-27" @default.
• W1997065559 title "Isotope effects in the infrared spectra of OCS–He complexes and clusters" @default.
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• W1997065559 doi "https://doi.org/10.1063/1.2356476" @default.
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