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• W2004334814 abstract "The formation mechanism and stability of silicon oxide clusters observed in the ablation of SiO targets at 266 nm were investigated by time-of-flight mass spectrometry, laser-induced fluorescence (LIF), and DFT calculations. Neutral and positively charged Sin+/0 and SinOmH0,1+ clusters were identified in the plume, but neutral SinOm could not be observed. The time distribution of SiO in the plume measured by postionization with an ArF laser (Δλ ≈ 1 nm, τ ≈ 14 ns) and mass spectrometric detection was compared with that obtained by LIF with narrowband dye laser selective excitation of one specific rovibronic transition in SiO. Postionization leads to a multicomponent distribution that extends up to times near 100 μs after ablation, whereas LIF measurements obtain time distributions shorter than 20 μs. DFT calculations of several SinOm0/+ were performed, showing that one photon absorption of the postionization laser makes available low-energy dissociation channels of the neutrals, whereas two photon absorption is required for ionization. DFT calculations were carried out for stoichiometric H-containing clusters SinOnH+ (n = 1−4). For n = 1,2, the optimized geometries involve bonding of hydrogen to one oxygen atom in the clusters; for n = 3 and 4, the structures containing H−Si bonds are more stable." @default.
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• W2004334814 date "2009-09-21" @default.
• W2004334814 modified "2023-10-17" @default.
• W2004334814 title "Silicon Oxide Cluster Formation and Stability in the Laser Ablation of SiO Targets" @default.
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• W2004334814 doi "https://doi.org/10.1021/jp906084p" @default.
• W2004334814 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/19810756" @default.
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