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• W2008610016 abstract "In this work we analyze Thermal Desorption Spectroscopy (TDS) experiments of gases considering simultaneously atomic diffusion in the bulk and recombinative reaction on the surface of a solid sample. We perform computer simulations in a three-dimensional cubic lattice, and compare the simulated spectra with numerical results from a simple reaction-diffusion model, and analytical results from models for the fast diffusion and fast reaction regimes. We analyze the effects on the spectra of each relevant parameter: diffusivity, reaction coefficient, heating rate, initial concentration of particles and sample size. We also develop a rate-limiting step identification procedure based on the analysis of peak position as a function of initial concentration. This last procedure applied to the simulations and to experimental TDS spectra produces very good results." @default.
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• W2008610016 date "1998-10-22" @default.
• W2008610016 modified "2023-10-18" @default.
• W2008610016 title "Bulk effects in Thermal Desorption Spectroscopy" @default.
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• W2008610016 doi "https://doi.org/10.1063/1.477261" @default.
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