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• W2023695171 startingPage "6642" @default.
• W2023695171 abstract "A large discrepancy exists among recent estimates of the primary quantum efficiencies (ϕ 1 ) of nitrogen dioxide photodecomposition, NO 2 + h ν → NO + O( 3 P ), in the wavelength range from 374 to 396 nm. To resolve this problem, quantum yields of formation of NO, O 2 , and NO 2 loss have been measured for NO 2 vapor at low pressures (0.13–0.30 torr) irradiated at selected wavelengths (334.1–404.3 nm) and temperatures (273–370 K). From these data, estimates of ϕ 1 were derived which confirm the previous findings of Jones and Bayes (1973 b ): ϕ 1 increases rapidly from near zero at 424 nm to near unity for excitation at λ < 394 nm. The temperature and wavelength dependences of ϕ 1 appear to be in qualitative accord with the simple theory of Pitts et al. (1964) that the energy deficiency for photodissociation of NO 2 excited at λ > 397.9 nm (λ diss ) is made up in large part from the rotational and vibrational energy of the NO 2 molecules. Recommended values for ϕ 1 based upon a review of these data and estimates made over a period of 58 years, are given as a function of wavelength." @default.
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• W2023695171 date "1987-06-20" @default.
• W2023695171 modified "2023-10-13" @default.
• W2023695171 title "Primary quantum yields of NO₂ photodissociation" @default.
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• W2023695171 doi "https://doi.org/10.1029/jd092id06p06642" @default.
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