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- W2027881475 abstract "Van der Waals-coupled materials, ranging from multilayers of graphene and MoS(2) to superlattices of nanoparticles, exhibit rich emerging behaviour owing to quantum coupling between individual nanoscale constituents. Double-walled carbon nanotubes provide a model system for studying such quantum coupling mediated by van der Waals interactions, because each constituent single-walled nanotube can have distinctly different physical structures and electronic properties. Here we systematically investigate quantum-coupled radial-breathing mode oscillations in chirality-defined double-walled nanotubes by combining simultaneous structural, electronic and vibrational characterizations on the same individual nanotubes. We show that these radial-breathing oscillations are collective modes characterized by concerted inner- and outer-wall motions, and determine quantitatively the tube-dependent van der Waals potential governing their vibration frequencies. We also observe strong quantum interference between Raman scattering from the inner- and outer-wall excitation pathways, the relative phase of which reveals chirality-dependent excited-state potential energy surface displacement in different nanotubes." @default.
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- W2027881475 date "2013-01-22" @default.
- W2027881475 modified "2023-10-12" @default.
- W2027881475 title "Quantum-coupled radial-breathing oscillations in double-walled carbon nanotubes" @default.
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- W2027881475 doi "https://doi.org/10.1038/ncomms2367" @default.
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