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- W2049512802 abstract "Activators generated by electron transfer atom transfer radical polymerization (AGET ATRP) of di(ethylene glycol) methyl ether methacrylate (M(EO)2MA) was successfully conducted in miniemulsion at 65 °C. The reaction system was stable without diffusion of monomer and polymer into the aqueous phase because the monomer is water-insoluble and PM(EO)2MA becomes hydrophobic above 25 °C. The polymerization was well-controlled with a mild water-soluble reducing agent, hydrazine, yielding PM(EO)2MA homopolymer with narrow molecular weight distribution (Mw/Mn = 1.2−1.6). Using this technique, well-defined PM(EO)2MA microgels were prepared with degradable disulfide cross-linker. The microgels became magnetic after physically loading oleic acid-coated Fe3O4 nanoparticles, which could not diffuse out of the microgels due to their hydrophobicity. Thermally responsive and drug loading−releasing behavior of the magnetic microgels was studied using Rhodamine B as a model for hydrophilic drugs. The drug releasing behavior can be well-controlled by both temperature and addition of reducing agent, indicating that the PM(EO)2MA magnetic microgels could find potential application for controlled targeted drug delivery." @default.
- W2049512802 created "2016-06-24" @default.
- W2049512802 creator A5015535709 @default.
- W2049512802 creator A5036993011 @default.
- W2049512802 creator A5056539244 @default.
- W2049512802 date "2009-08-07" @default.
- W2049512802 modified "2023-10-16" @default.
- W2049512802 title "Thermally Responsive PM(EO)<sub>2</sub>MA Magnetic Microgels via Activators Generated by Electron Transfer Atom Transfer Radical Polymerization in Miniemulsion" @default.
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- W2049512802 doi "https://doi.org/10.1021/cm901143e" @default.
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