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- W2055635055 abstract "An intense and stable continuous beam of S atoms and SO radicals is produced from a microwave discharge source operating in a SO2–He mixture. The S-atom beam, characterized by coupling mechanical velocity selection with magnetic analysis and detected by a quadrupole mass filter, has been employed in scattering experiments. The transmittance across a Stern–Gerlach magnetic selector, measured mass-spectrometrically at m/z=32 and 34 as a function of the beam velocity and of the deflecting field strength, indicates that the sulfur atoms are mainly in their electronic ground state 3Pj, with fine structure levels j=0, 1, 2 populated according to their degeneracies. Total integral cross-sections for collisions of S (3Pj) atoms with Ne, Ar, Kr and Xe have been measured in the beam velocity range 1.0–2.4 km s−1. The scattering data exhibit a glory interference effect with quenching of the amplitude of the glory pattern which increases along the rare-gas series from Ne to Xe. The results are analysed to yield a characterization of the spherical and anisotropic components of the interaction, providing lengths and strengths of the bonds in the six low lying states of the rare-gas sulfides NeS, ArS, KrS and XeS." @default.
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- W2055635055 date "2000-01-01" @default.
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- W2055635055 title "Production, characterization and scattering of a sulfur atom beam: Interatomic potentials for the rare-gas sulfides, RS (R = Ne, Ar, Kr, Xe)" @default.
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- W2055635055 doi "https://doi.org/10.1039/b001696i" @default.
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