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• W2059955764 abstract "The Fermi contact hyperfine interaction of hydrogen isotopes in liquid and solid water is below the vacuum value, shows a mass dependence, and has a negative temperature coefficient in the liquid. Furthermore, it shows a pronounced solvent isotope effect in H2O/D2O mixtures. This behavior is analyzed in terms of Dalgarno–Lewis perturbation theory for the atom in a spherical parabolic solvent potential and with a phenomenological model for spin delocalization onto solvent molecules. The results support previous suggestions that hydrogen atoms induce clathrate-like cages in liquid water. These may resemble the static structures of noble gas clathrates except that they are of transient dynamic nature in liquid water." @default.
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• W2059955764 date "1995-04-15" @default.
• W2059955764 modified "2023-10-17" @default.
• W2059955764 title "Isotope and temperature effects on the hyperfine interaction of atomic hydrogen in liquid water and in ice" @default.
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• W2059955764 doi "https://doi.org/10.1063/1.469333" @default.
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