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- W2063600047 abstract "A concise, enantiospecific synthesis of the phospholipase C inhibitor (−)-hispidospermidin (1) has been achieved by approximating the architecture of a reactive intermediate that may lie on the biosynthetic pathway leading to this natural product. Two compounds derived from (R)-(+)-pulegone were joined by a highly diastereoselective carbonyl addition. A proximity-facilitated, acid-induced bicyclization of spiro[4.5]deca-1,7-diene 29 gave rise to the tetracyclic framework of 1 and was the key transformation in this synthesis." @default.
- W2063600047 created "2016-06-24" @default.
- W2063600047 creator A5023114519 @default.
- W2063600047 creator A5078417346 @default.
- W2063600047 date "2003-08-01" @default.
- W2063600047 modified "2023-10-16" @default.
- W2063600047 title "A spontaneous bicyclization facilitates a synthesis of (−)-hispidospermidin" @default.
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- W2063600047 doi "https://doi.org/10.1016/s0040-4020(03)00936-0" @default.
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