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• W2071565327 abstract "Partial oxidation of methane to hydrogen and carbon monoxide (POM) over a Ni/TiO2 catalyst has been investigated using a fixed-bed reactor. Ni/TiO2 catalyst has high initial activity but undergoes deactivation during POM. Activation of methane on Ni/TiO2 was studied by employing a pulse reaction technique in the absence of gas phase oxygen. Methane pulse reactions demonstrate that the methane oxidation mechanism changes as the nickel oxidation state changes over Ni/TiO2. CH4 is efficiently oxidized into CO and H2 via a direct oxidation mechanism when Ni/TiO2 is reduced; while CH4 may be converted by a non-selective oxidation process over oxidized Ni/TiO2." @default.
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• W2071565327 date "2005-02-01" @default.
• W2071565327 modified "2023-09-27" @default.
• W2071565327 title "Partial oxidation of methane to hydrogen and carbon monoxide over a Ni/TiO2 catalyst" @default.
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• W2071565327 doi "https://doi.org/10.1016/j.molcata.2004.09.016" @default.
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