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- W2077648093 abstract "The first test of the information-theoretic approach to branching ratios has been made for the reaction: F + HD å HF† (V′, R′) + D å DF‡(V′, R′) + H. The vibrational (V′) and rotational (R′) product energy-distributions for both branches of this reaction have been obtained by the infrared chemiluminescence technique, and have been used in the calculation of an information-theoretic branching ratio, ΓHF/DF = 1.41 ± 0.18. This is in excellent agreement with the experimentally measured branching ratio of 1.45. However, results from classical trajectory calculations raise a question as to the significance of this agreement. Classical trajectory calculations (on various energy-surfaces) predict an increase in Γ with reagent J. The information-theoretic analysis applied to the product energy-distributions from these trajectory calculations leads to a qualitatively different result. As a possible alternative to the information-theoretic view, simple kinematic features are noted which could account for Γ > 1, as well as for the significant differences in product energy-distribution. On this alternative view, the two features are not indisolubly linked — the extent to which they appear in conjunction will depend on the nature of the energy surface." @default.
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- W2077648093 date "1976-01-01" @default.
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- W2077648093 title "An experimental test of the Bernstein—Levine theory of branching ratios" @default.
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- W2077648093 doi "https://doi.org/10.1016/0301-0104(76)80109-7" @default.
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