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- W2094779281 abstract "Abstract Two highly preorganized dizinc scaffolds based on compartmental pyrazolate ligands are found to incorporate 2‐azetidinone in its deprotonated β‐lactamide form as an N,O‐bridging ligand within the dimetallic pocket. Both dizinc β‐lactamide complexes 3· (ClO 4 ) 2 and 4· (ClO 4 ) 2 have been characterized structurally and spectroscopically, revealing a strengthening of the β‐lactamide C–N bond and a weakening of the C=O bond relative to free 2‐azetidinone. These findings contrast the reverse geometrical changes observed recently by Brombacher and Vahrenkamp for β‐lactamide N ‐bound to only a single zinc ion, thus underlining the particular dimetallic effect that is achieved by the cooperativity of two adjacent metal ions. (© Wiley‐VCH Verlag GmbH & Co. KGaA, 69451 Weinheim, Germany, 2005)" @default.
- W2094779281 created "2016-06-24" @default.
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- W2094779281 date "2005-06-01" @default.
- W2094779281 modified "2023-09-27" @default.
- W2094779281 title "Bridging β‐Lactam Coordination at Dinuclear Zinc Sites" @default.
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- W2094779281 doi "https://doi.org/10.1002/ejic.200401032" @default.
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