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• W2766585427 abstract "In this work, MgxFePO4 is exploited as a cathode material for rechargeable Mg-ion batteries. FePO4/C prepared via electrochemical delithiation of LiFePO4/C is directly used as the cathode in aqueous Mg2+ electrolyte, and reversible capacity is achieved for the first time. Notably, the capacity (82 mA h/g) is half of the theoretical value (164 mA h/g) and “asymmetric” discharge/charge behavior can be observed. In addition, first-principles calculations show it is the strong Mg-ion interactions between adjacent channels that not only limit the capacity of the cathode but also lead to the difference in rates for Mg-ion intercalation and deintercalation. This work provides experimental and theoretical evidence that reveal the mechanism of Mg-ion intercalation and deintercalation in a FePO4 host, which gives guidance in designing cathode materials for rechargeable batteries based on multivalent metal ions." @default.
• W2766585427 created "2017-11-10" @default.
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• W2766585427 date "2017-10-25" @default.
• W2766585427 modified "2023-10-17" @default.
• W2766585427 title "Olivine FePO₄ Cathode Material for Rechargeable Mg-Ion Batteries" @default.
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• W2766585427 doi "https://doi.org/10.1021/acs.inorgchem.7b02150" @default.
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