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• W2808752253 abstract "Abstract The molecular structures of CaO–FeO x –SiO 2 slags and their inorganic polymer counterparts were determined using neutron and X‐ray scattering with subsequent pair distribution function ( PDF ) analysis. The slags were synthesized with approximate molar compositions: 0.17CaO–0.83FeO–SiO 2 and 0.33CaO–0.67FeO–SiO 2 (referred to as low‐Ca and high‐Ca, respectively) . The PDF data on the slags reasserted the predominantly glassy nature of this iron‐rich industrial byproduct. The dominant metal‐metal correlation was Fe–Si (3.20‐3.25 Å), with smaller contributions from Fe–Ca (3.45‐3.50 Å) and Fe–Fe (2.95‐3.00 Å). After inorganic polymer synthesis, a rise in the amount of Fe 3+ was observed via the shift of the Fe–O bond length to shorter distances. This shortening of the Fe–O distance in the binder is also evidenced by the apparent rise of the Fe–Fe correlation at 2.95‐3.00 Å, although this feature may also suggest a potential aggregation of FeO x clusters. In general, the atomic arrangements of the reaction product was shown to be very similar to the precursor structure and the dominance of the Fe–Si correlation suggests the participation of Fe in the silicate network. The binder was shown to be glassy, as no distinct atom‐atom correlations were observed beyond 8 Å." @default.
• W2808752253 created "2018-06-29" @default.
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• W2808752253 date "2018-06-28" @default.
• W2808752253 modified "2023-10-05" @default.
• W2808752253 title "Molecular structure of CaO–FeO _x –SiO ₂ glassy slags and resultant inorganic polymer binders" @default.
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• W2808752253 doi "https://doi.org/10.1111/jace.15880" @default.
• W2808752253 hasPublicationYear "2018" @default.
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