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• W2912523060 startingPage "1384" @default.
• W2912523060 abstract "A concise approach to synthesize the tetracyclic framework of the marine diterpenoid plumisclerin A is described. Starting from commercially available iridoid genipin, a highly selective intermolecular Diels-Alder reaction was utilized to construct the A/B/C tricycle. Later, a four-step sequence involving stereoselective epoxidation and Dauben oxidative rearrangement was developed to introduce the requisite enone moiety. The unique tricyclo[4,3,1,01,5]decane motif was successfully forged via a late-stage SmI2-mediated reductive coupling." @default.
• W2912523060 created "2019-02-21" @default.
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• W2912523060 date "2019-02-15" @default.
• W2912523060 modified "2023-10-18" @default.
• W2912523060 title "Synthetic Studies toward Plumisclerin A" @default.
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• W2912523060 doi "https://doi.org/10.1021/acs.orglett.9b00095" @default.
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