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• W2913184679 abstract "We present the magnetic structure of $mathrm{TmMn_3O_6}$, solved via neutron powder diffraction - the first such study of any $Rmathrm{Mn_3O_6}$ A-site columnar-ordered quadruple perovskite to be reported. We demonstrate that long range magnetic order develops below 74 K, and at 28 K a spin-flop transition occurs driven by $f$-$d$ exchange and rare earth single ion anisotropy. In both magnetic phases the magnetic structure may be described as a collinear ferrimagnet, contrary to conventional theories of magnetic order in the manganite perovskites. Instead, we show that these magnetic structures can be understood to arise due to ferro-orbital order, the A, A$'$ and A$''$ site point symmetry, $mm2$, and the dominance of A-B exchange over both A-A and B-B exchange, which together are unique to the $Rmathrm{Mn_3O_6}$ perovskites." @default.
• W2913184679 created "2019-02-21" @default.
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• W2913184679 date "2019-03-21" @default.
• W2913184679 modified "2023-09-27" @default.
• W2913184679 title "Magnetic structure and spin-flop transition in the <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mi>A</mml:mi></mml:math> -site columnar-ordered quadruple perovskite <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mrow><mml:msub><mml:mi>TmMn</mml:mi><mml:mn>3</mml:mn></mml:msub><mml:msub><mml:mi mathvariant=normal>O</mml:mi><mml:mn>6</mml:mn></mml:msub></mml:mrow></mml:math>" @default.
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• W2913184679 doi "https://doi.org/10.1103/physrevb.99.104424" @default.
• W2913184679 hasPublicationYear "2019" @default.
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