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- W3000694291 abstract "Abstract Fe-oxide/Al2O3 catalysts were fabricated by depositing Fe-oxide nanoparticles with a lateral size less than ~2 nm in a highly dispersed manner within mesoporous Al2O3 using temperature-regulated chemical vapor deposition (TRCVD). The Fe-oxide/Al2O3 catalysts were post-annealed at either 450 °C (for 2 h) or 750 °C (for 2 or 8 h) and were used to catalyze NO reduction by CO. Catalytic activity was significantly enhanced with increased annealing temperature and time. Secondary ion mass spectrometry using Bi3+ as the primary ion shows an increase in the FeAlO+ signal from the interfaces between Fe-oxide and Al2O3 with increasing annealing temperature and time, suggesting that the enhanced interaction between Al2O3 and Fe-oxide is responsible for the increased catalytic activity. It is shown that TRCVD with a proper post-annealing step is a competitive tool for preparation of heterogeneous catalysts with highly dispersed catalyst nanostructures within mesoporous substrates that contain rich oxide/oxide interfaces and allow enhanced catalytic activity." @default.
- W3000694291 created "2020-01-23" @default.
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- W3000694291 date "2020-04-01" @default.
- W3000694291 modified "2023-09-24" @default.
- W3000694291 title "Reduction of NO by CO catalyzed by Fe-oxide/Al2O3: Strong catalyst-support interaction for enhanced catalytic activity" @default.
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- W3000694291 doi "https://doi.org/10.1016/j.apsusc.2020.145300" @default.
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