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- W3003079780 abstract "This study aims to investigate the photothermal oxidation removal of Hg0 in simulated flue gases using photothermal catalysts at relatively low temperatures of 120–160 °C in two phases: the first phase applied the sol–gel method to prepare TiO2 and CeO2/TiO2 photothermal catalysts and characterized surface properties by specific surface area analysis, X-ray diffraction, X-ray photoelectron spectroscopy (XPS), and photoluminescence spectroscopy. The second phase investigated the effects of operating parameters on Hg0 oxidation efficiency at lower temperatures of 100–160 °C. The operating parameters included reaction temperatures and modified concentrations of CeO2. Experimental results indicated that TiO2 prepared by the sol–gel method was mainly in the anatase phase. XPS analysis showed that Ce mostly existed in the form of Ce4+. The content of surface-chemisorbed oxygen increased with the modification amount of CeO2. Photothermal catalytic oxidation results indicated that CeO2/TiO2 had a much higher oxidation efficiency of Hg0 at 120–160 °C than neat TiO2, which increased from 30–60 to >90%. 7%CeO2/TiO2 not only had the best photothermal performance but also maintained high efficiency at a relatively higher reaction temperature of 160 °C." @default.
- W3003079780 created "2020-01-30" @default.
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- W3003079780 date "2020-01-21" @default.
- W3003079780 modified "2023-09-28" @default.
- W3003079780 title "Enhancement of Oxidation Efficiency of Elemental Mercury by CeO<sub>2</sub>/TiO<sub>2</sub> at Low Temperatures Governed by Different Mechanisms" @default.
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- W3003079780 doi "https://doi.org/10.1021/acsomega.9b02897" @default.
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