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• W4205185963 abstract "Fluorescence spectroscopy can provide high-level chemical characterization and quantification that is suitable for use in online process monitoring and control. However, the high-dimensionality of excitation-emission matrices and superposition of underlying signals is a major challenge to implementation. Herein the use of Convolutional Neural Networks (CNNs) is investigated to interpret fluorescence spectra and predict the formation of disinfection by-products during drinking water treatment. Using deep CNNs, mean absolute prediction error on a test set of data for total trihalomethanes, total haloacetic acids, and the major individual species were all < 6 µg/L and represent a significant difference improved by 39-62% compared to multi-layer perceptron type networks. Heat maps that identify spectral areas of importance for prediction showed unique humic-like and protein-like regions for individual disinfection by-product species that can be used to validate models and provide insight into precursor characteristics. The use of fluorescence spectroscopy coupled with deep CNNs shows promise to be used for rapid estimation of DBP formation potentials without the need for extensive data pre-processing or dimensionality reduction. Knowledge of DBP formation potentials in near real-time can enable tighter treatment controls and management efforts to minimize the exposure of the public to DBPs." @default.
• W4205185963 created "2022-01-26" @default.
• W4205185963 creator A5026926340 @default.
• W4205185963 date "2022-01-12" @default.
• W4205185963 modified "2023-10-07" @default.
• W4205185963 title "Application of convolutional neural networks for prediction of disinfection by-products" @default.
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• W4205185963 doi "https://doi.org/10.1038/s41598-021-03881-w" @default.
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