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- W4283453178 abstract "Abstract Graphitic carbon nitride (g-C 3 N 4 ) has attracted much attention due to its unique polymeric structure of carbon and nitrogen in the form of heptazine units. In this study, a nickel catalyst supported on graphitic carbon nitride was prepared by a facile impregnation method. Ni/g-C 3 N 4 desorption and reduction behaviour with carbon monoxide (CO) was investigated by temperature-programmed desorption (TPD) and reduction (TPR). The as-prepared Ni/g-C 3 N 4 catalyst was also characterized by X-ray diffraction (XRD), N 2 physisorption, and X-ray photoelectron spectroscopy (XPS). It was found that the utilization of g-C 3 N 4 as a catalyst support enhances the complete reduction of Ni species and CO desorption. This can be attributed to the role of g-C 3 N 4 support as a reducing agent for Ni, as well as its basicity owing to the richness of nitrogen functional group. The good performance of Ni/g-C 3 N 4 catalyst towards CO methanation can be ascribed to the improvement in adsorption and activation of CO molecules on the active sites and the number of surface basic sites." @default.
- W4283453178 created "2022-06-26" @default.
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- W4283453178 date "2022-06-24" @default.
- W4283453178 modified "2023-10-16" @default.
- W4283453178 title "Carbon Monoxide Desorption and Reduction Studies of Graphitic Carbon Nitride Supported Nickel Catalysts for CO Methanation" @default.
- W4283453178 doi "https://doi.org/10.21203/rs.3.rs-1736656/v1" @default.
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