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• W1988366956 abstract "Nickelates ANiO3 (A=Pr, Nd, Sm, Lu, Y, Tl) containing Mössbauer probe 57Fe atoms were synthesized. In the case of nickelates with larger rare earth (A=Pr, Nd, Sm) the Mössbauer spectra confirm that ferric ions are located in single type of crystallographic positions. On the contrary, the spectra of ANi0.98Fe0.02O3 with small cations (A=Lu, Y, Tl) can be described as a superposition of two sub-spectra which indicate that 57Fe probe atoms are simultaneously stabilized in two non-equivalent crystallographic positions. These results have been interpreted in terms of partial charge disproportionation of Ni3+ cations associated with the electronic localization in monoclinic distorted Lu, Y, Tl nickelates. The modification of 57Fe spectra for TlNi0.98Fe0.02O3 as a function of temperature has shown that this charge disproportionation occurs in varying degrees, corresponding to the charge states Fe(3+σ)+ and Fe(3−σ′)+. On the contrary, the spectra for Lu and Y nickelates show that charge variation (σ,σ′) for dopant Fe(1) and Fe(2) cations does not depend on temperature." @default.
• W1988366956 created "2016-06-24" @default.
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• W1988366956 date "2002-10-01" @default.
• W1988366956 modified "2023-10-13" @default.
• W1988366956 title "Mossbauer Investigation of 57Fe-Doped Ni(III) Perovskites ANi0.98Fe0.02O3 (A=Pr, Nd, Sm, Y, Lu, Tl) versus Temperature" @default.
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• W1988366956 doi "https://doi.org/10.1006/jssc.2002.9699" @default.
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