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• W1997221570 endingPage "61" @default.
• W1997221570 startingPage "54" @default.
• W1997221570 abstract "We investigated the local atomic and electronic structures of two related systematic sets of ternary uranium oxides, NaUO3–KUO3–RbUO3 and BaUO3–Ba2U2O7–BaUO4, by measuring the X-ray absorption near edge structure (XANES). The results are compared with calculations based on a self-consistent real space full multiple scattering analysis. We found a very good agreement between measured and calculated spectra, which indicates that the uranium ions are in a pure U5+ oxidation state in these compounds. The low energy shoulder observed in the U L3 edge XANES is an intrinsic feature of the uranium unoccupied 6d electronic states of the U5+ ions within the studied materials. Specific double shoulder features in the higher energy range of the U L3 edge XANES can be interpreted as indicative of the pure cubic perovskite structure." @default.
• W1997221570 created "2016-06-24" @default.
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• W1997221570 date "2007-01-01" @default.
• W1997221570 modified "2023-09-27" @default.
• W1997221570 title "Local structure and oxidation state of uranium in some ternary oxides: X-ray absorption analysis" @default.
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• W1997221570 doi "https://doi.org/10.1016/j.jssc.2006.08.038" @default.
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