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• W2005702991 abstract "In the present paper, we examine how H sorption should depend on the cathodic H2 evolution mechanism, through the potential dependence of the fractional coverage by adsorbed H. The states of adsorbed and absorbed H are treated in terms of site-fraction statistics in order to determine the chemical potentials of the adsorbed and absorbed H. Then, the relationships to the overpotential in the H2 evolution reaction are derived and the efficiency of H sorption in relation to the coevolution of H2 (important for metal hydride battery electrode charging) can be examined in terms of reaction mechanisms. Difficulties arising with application of the Nernst equation to H sorption when appreciable overpotentials for H2 evolution are involved, i.e. at appreciable cathodic current densities, are examined. Finally, the interesting effects of ‘catalyst poisons’, which promote H sorption into host metals, are examined in terms of the effects of competitive adsorption between the poison and H at the surface. Conventional ideas about these effects are inconsistent with information on the diminution of H coverage caused by competitive adsorption of poisons; alternative mechanisms are discussed and a new surface-thermodynamic basis for the enhancement of H sorption by adsorbed poisons is proposed." @default.
• W2005702991 created "2016-06-24" @default.
• W2005702991 creator A5022922272 @default.
• W2005702991 creator A5089825488 @default.
• W2005702991 date "1993-10-01" @default.
• W2005702991 modified "2023-09-23" @default.
• W2005702991 title "Thermodynamic and electrode kinetic factors in cathodic hydrogen sorption into metals and its relationship to hydrogen adsorption and poisoning" @default.
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• W2005702991 doi "https://doi.org/10.1016/0022-0728(93)80373-p" @default.
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