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• W2022047868 abstract "We calculate the ion distributions around an interface in fluid mixtures of highly polar and less polar fluids (water and oil) for two and three ion species. We take into account the solvation and image interactions between ions and solvent. We show that hydrophilic and hydrophobic ions tend to undergo a microphase separation at an interface, giving rise to an enlarged electric double layer. We also derive a general expression for the surface tension of electrolyte systems, which contains a negative electrostatic contribution proportional to the square root of the bulk salt density. The amplitude of this square-root term is small for hydrophilic ion pairs but is much increased for hydrophilic and hydrophobic ion pairs. For three ion species, including hydrophilic and hydrophobic ions, we calculate the ion distributions to explain those obtained by x-ray reflectivity measurements." @default.
• W2022047868 created "2016-06-24" @default.
• W2022047868 creator A5080902652 @default.
• W2022047868 date "2008-06-12" @default.
• W2022047868 modified "2023-09-27" @default.
• W2022047868 title "Surface tension of electrolytes: Hydrophilic and hydrophobic ions near an interface" @default.
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• W2022047868 doi "https://doi.org/10.1063/1.2936992" @default.
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