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• W2025707959 abstract "It is shown how exact formulas for the longitudinal and transverse dielectric correlation times and complex polarizability tensor, of a single axis rotator with two equivalent sites may be found. This is accomplished by writing the Laplace transforms of the dipole autocorrelation functions as three term recurrence relations and solving them in terms of continued fractions. The solution of these recurrence relations, in the zero frequency limit, yields the correlation times in terms of modified Bessel functions of the first kind. The previous result of Lauritzen and Zwanzig for the longitudinal relaxation time, based on an asymptotic expansion of the Sturm–Liouville equation, is regained in the limit of high potential barriers." @default.
• W2025707959 created "2016-06-24" @default.
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• W2025707959 date "1993-09-01" @default.
• W2025707959 modified "2023-09-25" @default.
• W2025707959 title "Exact solution for the correlation times of dielectric relaxation of a single axis rotator with two equivalent sites" @default.
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• W2025707959 doi "https://doi.org/10.1063/1.466097" @default.
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