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- W2029133059 abstract "A theory of optical echo spectroscopies of large polyatomic molecules in condensed phases is developed. Using phase space correlation functions, we examine the interrelationships among the following optical measurements: ordinary photon echo, stimulated photon echo, accumulated photon echo, incoherent accumulated photon echo, and pump–probe absorption. Conditions for the elimination of inhomogeneous broadening in these experiments are specified. A multimode Brownian oscillator model is used to account for high frequency molecular vibrations, as well as solvent modes, and electronic dephasing processes. The effects of quantum beats, spectral diffusion, and homogeneous dephasing on the echo signals are studied and compared in detail with pump–probe and hole burning spectroscopy." @default.
- W2029133059 created "2016-06-24" @default.
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- W2029133059 date "1991-01-01" @default.
- W2029133059 modified "2023-09-25" @default.
- W2029133059 title "Photon echoes of polyatomic molecules in condensed phases" @default.
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- W2029133059 doi "https://doi.org/10.1063/1.460376" @default.
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