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- W2031462293 abstract "Dips appearing in the L-edge total fluorescence yield (TFY) spectra of transition-metal ions in aqueous solutions have been recently attributed to, orbital mixing of the solute with the solvent orbitals. Here we compare the L-edge TFY, Oxygen Kα and Co2+ Ll(3s → 2p3/2), Lη(3s → 2p1/2), Lα(3d → 2p3/2) and Lβ(3d → 2p1/2) –edge partial fluorescence yield with the transmission spectrum. We thereby confirm that these mixed orbitals lead to electron delocalization between the valence d-orbitals of the transition metal and the valence bands of the solvent molecules, quenching their X-ray fluorescence." @default.
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- W2031462293 date "2012-09-01" @default.
- W2031462293 modified "2023-10-17" @default.
- W2031462293 title "On the origin of dips in total fluorescence yield X-ray absorption spectra: Partial and inverse partial fluorescence yield at the L-edge of cobalt aqueous solution" @default.
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- W2031462293 doi "https://doi.org/10.1016/j.cplett.2012.07.067" @default.
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