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• W2048366968 endingPage "12" @default.
• W2048366968 startingPage "4" @default.
• W2048366968 abstract "The aim of this study is to understand the sorption of tributyltin (TBT) onto natural quartz sand by classical batch experiments and spectroscopic surface analyses. At pH<6, the major species of TBT is the cation TBT(+). Due to the presence of both the cationic part and the butyl chains, TBT should present amphiphilic properties. For concentrations lower than 40 microM, TBT sorption occurs as a homovalent 1:1 cation exchange between either H(+) or Na(+) and TBT(+). The increasing affinity of TBT with respect to the different materials follows the series kaolinite<<natural sand<treated sand<pure quartz. From XPS analyses, where the chemical environment of Sn did not change, indicating possible complete reversibility of the TBT sorption, it seems that inner-sphere surface complexes could be formed due to the increase in the 3d-level binding energy. At TBT concentrations higher than 100 microM, we showed by flotation experiments and XPS analysis that the surface becomes hydrophobic. After one monolayer was formed, the TBT sorption could thus be due to hydrophobic interaction between the butyl chains of the sorbed TBT and those of the TBT still available from the bulk solution. This mechanism is consistent with surface condensation and the shape of the sorption isotherm." @default.
• W2048366968 created "2016-06-24" @default.
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• W2048366968 date "2003-07-01" @default.
• W2048366968 modified "2023-10-12" @default.
• W2048366968 title "Sorption of tributyltin onto a natural quartz sand" @default.
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• W2048366968 doi "https://doi.org/10.1016/s0021-9797(03)00238-8" @default.
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• W2048366968 hasPublicationYear "2003" @default.
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