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• W2081443389 abstract "The high-temperature reaction of NO with H2 has been studied behind reflected shock waves in the temperature range of 1760–2160 K at total pressures of 1.4 to 2.0 bar by monitoring the time-dependent H-atom concentrations in the postshock reaction zone using atomic resonance absorption spectroscopy (ARAS). Mixtures of NO and H2 highly diluted in argon were used as initial reactants. The rate coefficient, k1, of the initiation reaction: NO + H2 → HNO + H has been determined from the measured initial H-atom concentration slopes to be k1 = 1.5 × 1013 exp(−26165K/T)cm3 mol−1 s−1, taking the fast decomposition of HNO into account. This direct deterination of the rate coefficient k1 was possible, because the contribution of H2 dissociation to the total H atom concentration of the system was relatively small in the temperature and concentration ranges of this study. Measured O-atom concentrations in the high-temperature H2/NO/Ar reaction system (2560 K ≤ T ≤ 4040 K) were sensitive to the reaction NO + H → OH + N, resulting in an estimate of its rate coefficient. A simplified mechanism of 15 elementary reactions was able to predict all measured H and O atom profiles with reasonable accuracy." @default.
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• W2081443389 date "1994-12-01" @default.
• W2081443389 modified "2023-10-11" @default.
• W2081443389 title "A shock tube study of the reaction H2 + NO → HNO + H" @default.
• W2081443389 cites W1978168565 @default.
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• W2081443389 doi "https://doi.org/10.1016/0010-2180(94)90054-x" @default.
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