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- W2296908622 abstract "Abstract Graphene nanoribbons display extraordinary optical properties due to one-dimensional quantum-confinement, such as width-dependent bandgap and strong electron–hole interactions, responsible for the formation of excitons with extremely high binding energies. Here we use femtosecond transient absorption spectroscopy to explore the ultrafast optical properties of ultranarrow, structurally well-defined graphene nanoribbons as a function of the excitation fluence, and the impact of enhanced Coulomb interaction on their excited states dynamics. We show that in the high-excitation regime biexcitons are formed by nonlinear exciton–exciton annihilation, and that they radiatively recombine via stimulated emission. We obtain a biexciton binding energy of ≈250 meV, in very good agreement with theoretical results from quantum Monte Carlo simulations. These observations pave the way for the application of graphene nanoribbons in photonics and optoelectronics." @default.
- W2296908622 created "2016-06-24" @default.
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- W2296908622 date "2016-03-17" @default.
- W2296908622 modified "2023-09-25" @default.
- W2296908622 title "Exciton–exciton annihilation and biexciton stimulated emission in graphene nanoribbons" @default.
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- W2296908622 doi "https://doi.org/10.1038/ncomms11010" @default.
- W2296908622 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/4800436" @default.
- W2296908622 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/26984281" @default.
- W2296908622 hasPublicationYear "2016" @default.
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