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- W2765646140 abstract "A one-step straightforward strategy has been developed to incorporate free imidazole molecules into a highly stable metal-organic framework (NENU-3, ([Cu12(BTC)8(H2O)12][HPW12O40])·Guest). The resulting material Im@(NENU-3) exhibits a very high proton conductivity of 1.82 × 10-2 S cm-1 at 90% RH and 70 °C, which is significantly higher than 3.16 × 10-4 S cm-1 for Im-Cu@(NENU-3a) synthesized through a two-step approach with mainly terminal bound imidazole molecules inside pores. Single crystal structure reveals that imidazole molecules in Im-Cu@(NENU-3a) isolate lattice water molecules and then block proton transport pathway, whereas high concentration of free imidazole molecules within Im@(NENU-3) significantly facilitate successive proton-hopping pathways through formation of hydrogen bonded networks." @default.
- W2765646140 created "2017-11-10" @default.
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- W2765646140 date "2017-10-31" @default.
- W2765646140 modified "2023-10-17" @default.
- W2765646140 title "Straightforward Loading of Imidazole Molecules into Metal–Organic Framework for High Proton Conduction" @default.
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- W2765646140 doi "https://doi.org/10.1021/jacs.7b09163" @default.
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