FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W2778565536> ?p ?o ?g. }

• W2778565536 endingPage "332" @default.
• W2778565536 startingPage "323" @default.
• W2778565536 abstract "In this study, batch experiments were carried out to investigate the key factors on sulfamethoxazole (SMX) removal kinetics in a new AOPs based on the combination of zero valent iron (Fe0) and bisulfite (S(IV)). With the increase of Fe0 from 0.25 mM to 5 mM, the removal rate of SMX was linearly increased in the Fe0/S(IV)/O2 system by accelerating the activation of S(IV) and Fe0 corrosion to accelerate. In the first 10 min of reaction, the increasing concentration of S(IV) inhibited SMX removal after since the high S(IV) concentration quenched reactive oxidative species (ROS). Then SMX removal rate was accelerated with the increase of S(IV) concentration after S(IV) were consumed up. The optimal ratio of S(IV) concentrations to Fe0 concentration for SMX removal in the Fe0/S(IV)/O2 system was 1:1. With SMX concentrations increasing from 1 to 50 μM, SMX removal rate was inhibited for the limitation of ROS yields. Although the presence of SO4- and OH was confirmed by electron paramagnetic resonance (EPR) spectrum, OH was identified as the dominant ROS in the Fe0/S(IV)/O2 system by chemical quenching experiments. Besides, strong inhibitive effects of 1,10-phenanthroline on SMX degradation kinetics by Fe0/S(IV)/O2 proved that the generation of ROS was rely on the release of Fe(II) and Fe(III). The generation of SO4- was ascribed to the activation of S(IV) by Fe(II)/Fe(III) recycling and the activation of HSO5- by Fe(II). And OH was simultaneously transformed from SO4- and generated by Fe0/O2. Density functional theory (DFT) calculation was conducted to reveal special reactive sites on SMX for radicals attacking and predicted intermediates. Finally, four possible SMX degradation pathways were accordingly proposed in the Fe0/S(IV)/O2 system based on experimental methods and DFT calculation." @default.
• W2778565536 created "2018-01-05" @default.
• W2778565536 creator A5016518424 @default.
• W2778565536 creator A5023716546 @default.
• W2778565536 creator A5041498647 @default.
• W2778565536 creator A5041800896 @default.
• W2778565536 creator A5047208840 @default.
• W2778565536 creator A5056623822 @default.
• W2778565536 creator A5061195656 @default.
• W2778565536 creator A5088589059 @default.
• W2778565536 date "2018-07-01" @default.
• W2778565536 modified "2023-10-10" @default.
• W2778565536 title "Hydroxyl radical dominated degradation of aquatic sulfamethoxazole by Fe0/bisulfite/O2: Kinetics, mechanisms, and pathways" @default.
• W2778565536 cites W1926950498 @default.
• W2778565536 cites W1958791145 @default.
• W2778565536 cites W1964754775 @default.
• W2778565536 cites W1968329395 @default.
• W2778565536 cites W1973123407 @default.
• W2778565536 cites W1974355116 @default.
• W2778565536 cites W1983228601 @default.
• W2778565536 cites W2006809388 @default.
• W2778565536 cites W2013731232 @default.
• W2778565536 cites W2014960268 @default.
• W2778565536 cites W2025877903 @default.
• W2778565536 cites W2038173949 @default.
• W2778565536 cites W2045185797 @default.
• W2778565536 cites W2049272618 @default.
• W2778565536 cites W2053322034 @default.
• W2778565536 cites W2063042339 @default.
• W2778565536 cites W2071955309 @default.
• W2778565536 cites W2075039454 @default.
• W2778565536 cites W2076531055 @default.
• W2778565536 cites W2084029513 @default.
• W2778565536 cites W2086176473 @default.
• W2778565536 cites W2086498245 @default.
• W2778565536 cites W2086841044 @default.
• W2778565536 cites W2088651962 @default.
• W2778565536 cites W2091712457 @default.
• W2778565536 cites W2095131012 @default.
• W2778565536 cites W2095227392 @default.
• W2778565536 cites W2099298633 @default.
• W2778565536 cites W2102237276 @default.
• W2778565536 cites W2120512121 @default.
• W2778565536 cites W2127925117 @default.
• W2778565536 cites W2132525235 @default.
• W2778565536 cites W2142102316 @default.
• W2778565536 cites W2207387449 @default.
• W2778565536 cites W2236556070 @default.
• W2778565536 cites W2312293937 @default.
• W2778565536 cites W2320541794 @default.
• W2778565536 cites W2324202036 @default.
• W2778565536 cites W2335221168 @default.
• W2778565536 cites W2398795347 @default.
• W2778565536 cites W2405376438 @default.
• W2778565536 cites W2413402613 @default.
• W2778565536 cites W2565589777 @default.
• W2778565536 cites W2568273126 @default.
• W2778565536 cites W25881410 @default.
• W2778565536 cites W2600473920 @default.
• W2778565536 cites W2603383502 @default.
• W2778565536 cites W2767380710 @default.
• W2778565536 cites W2949613746 @default.
• W2778565536 cites W4256603424 @default.
• W2778565536 doi "https://doi.org/10.1016/j.watres.2017.12.046" @default.
• W2778565536 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/29627708" @default.
• W2778565536 hasPublicationYear "2018" @default.
• W2778565536 type Work @default.
• W2778565536 sameAs 2778565536 @default.
• W2778565536 citedByCount "204" @default.
• W2778565536 countsByYear W27785655362018 @default.
• W2778565536 countsByYear W27785655362019 @default.
• W2778565536 countsByYear W27785655362020 @default.
• W2778565536 countsByYear W27785655362021 @default.
• W2778565536 countsByYear W27785655362022 @default.
• W2778565536 countsByYear W27785655362023 @default.
• W2778565536 crossrefType "journal-article" @default.
• W2778565536 hasAuthorship W2778565536A5016518424 @default.
• W2778565536 hasAuthorship W2778565536A5023716546 @default.
• W2778565536 hasAuthorship W2778565536A5041498647 @default.
• W2778565536 hasAuthorship W2778565536A5041800896 @default.
• W2778565536 hasAuthorship W2778565536A5047208840 @default.
• W2778565536 hasAuthorship W2778565536A5056623822 @default.
• W2778565536 hasAuthorship W2778565536A5061195656 @default.
• W2778565536 hasAuthorship W2778565536A5088589059 @default.
• W2778565536 hasConcept C104317684 @default.
• W2778565536 hasConcept C121332964 @default.
• W2778565536 hasConcept C121745418 @default.
• W2778565536 hasConcept C139066938 @default.
• W2778565536 hasConcept C13965031 @default.
• W2778565536 hasConcept C148898269 @default.
• W2778565536 hasConcept C150194340 @default.
• W2778565536 hasConcept C150394285 @default.
• W2778565536 hasConcept C178790620 @default.
• W2778565536 hasConcept C179104552 @default.
• W2778565536 hasConcept C185592680 @default.
• W2778565536 hasConcept C187961010 @default.
• W2778565536 hasConcept C190727270 @default.
• W2778565536 hasConcept C2775959680 @default.

• next