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- W2780457624 abstract "We study the effects of higher-order electronic correlations in the systems with particle-hole excited states using a relativistic hybrid method that combines configuration interaction and linearized coupled-cluster approaches. We find the configuration interaction part of the calculation sufficiently complete for eight electrons while maintaining good quality of the effective coupled-cluster potential for the core. Excellent agreement with experiment was demonstrated for a test case of ${mathrm{La}}^{3+}$. We apply our method for homolog actinide ions ${mathrm{Th}}^{4+}$ and ${mathrm{U}}^{6+}$ which are of experimental interest due to a puzzle associated with the resonant excitation Stark ionization spectroscopy method. These ions are also of interest to actinide chemistry." @default.
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- W2780457624 date "2018-01-25" @default.
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- W2780457624 title "Atomic properties of actinide ions with particle-hole configurations" @default.
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- W2780457624 doi "https://doi.org/10.1103/physreva.97.012511" @default.
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