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- W2801974040 abstract "Photon-induced fragmentation of a full set of chlorinated methanes (CH3Cl, CH2Cl2, CHCl3, CCl4) has been investigated both experimentally and computationally. Using synchrotron radiation and electron-ion coincidence measurements, the dissociation processes were studied after chlorine 2p electron excitation. Experimental evidence for CH3Cl and CH2Cl2 contains unique features suggesting that fast dissociation processes take place. By contrast, CHCl3 and CCl4 molecules do not contain the same features, hinting that they experience alternative mechanisms for dissociation and charge migration. Computational work indicates differing rates of charge movement after the core-excitation, which can be used to explain the differences observed experimentally." @default.
- W2801974040 created "2018-05-17" @default.
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- W2801974040 date "2018-05-02" @default.
- W2801974040 modified "2023-10-08" @default.
- W2801974040 title "Role of ultrafast dissociation in the fragmentation of chlorinated methanes" @default.
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- W2801974040 doi "https://doi.org/10.1063/1.5026720" @default.
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