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- W2894456436 abstract "Organic carboxyl compounds are promising anode candidates for lithium ion batteries in which oxygen-related redox dominates the reaction mechanisms. Herein, two nanostructured organic electrodes of π-extended naphthyl-based dicarboxylate and dithiocarboxylate compounds, namely sodium naphthalene-2,6-dicarboxylate (SND) and sodium naphthalene-2,6-bis(carbothioate) (SNB) are first synthesized and investigated systematically for lithium ion battery. Through introducing less electronegative sulfur atoms into carboxylic groups at molecular level, SNB exhibits a different voltage profile and delivers higher reversible capacity of 280 mAh g-1 than SND (198 mAh g-1) at a current density of 50 mA g-1. A combination of electrochemical properties and DFT calculations reveals that SNB could reversibly store three Li+ per formula unit, while SND only stores two Li+. The present work offers a new strategy to develop redox molecules with tunable redox potentials and accommodation more alkaline ions for high performance battery systems." @default.
- W2894456436 created "2018-10-05" @default.
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- W2894456436 date "2018-09-25" @default.
- W2894456436 modified "2023-10-17" @default.
- W2894456436 title "Three-Electron Redox Enabled Dithiocarboxylate Electrode for Superior Lithium Storage Performance" @default.
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- W2894456436 doi "https://doi.org/10.1021/acsami.8b11485" @default.
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