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• W2899684319 abstract "Photocatalytic conversion of diluted CO2 into solar fuel is highly appealing yet still in its infancy. Herein, we demonstrate the metal-node-dependent performance for photoreduction of diluted CO2 by constructing Ni metal-organic framework (MOF) monolayers (Ni MOLs). In diluted CO2 (10 %), Ni MOLs exhibit a highest apparent quantum yield of 1.96 % with a CO selectivity of 96.8 %, which not only exceeds reported systems in diluted CO2 but also is superior to most catalysts in pure CO2 . Whereas isostructural Co MOLs is almost inactive in diluted CO2 , indicating the performance is dependent on the metal nodes. Experimental and theoretical investigations show that strong CO2 binding affinity of Ni MOLs is the crucial factor, which stabilizes the Ni-CO2 adducts and facilitates CO2 -to-CO conversion." @default.
• W2899684319 created "2018-11-16" @default.
• W2899684319 creator A5008893402 @default.
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• W2899684319 date "2018-12-17" @default.
• W2899684319 modified "2023-10-17" @default.
• W2899684319 title "Nickel Metal–Organic Framework Monolayers for Photoreduction of Diluted CO ₂ : Metal‐Node‐Dependent Activity and Selectivity" @default.
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• W2899684319 doi "https://doi.org/10.1002/anie.201811545" @default.
• W2899684319 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30402925" @default.
• W2899684319 hasPublicationYear "2018" @default.
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