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- W2900858045 abstract "A simple and efficient method for the adsorption and immobilization of the radioactive ionic-corrosion-products Co2+, Cr3+, Mn2+, Fe2+, Ni2+, Cu2+ and Zn2+ generated in nuclear reactor coolant has been developed using a magnetic hydroxyapatite nanocomposite (MA-HAP) and a cold-sintering technique. The structure, morphology, magnetic properties and zeta potential of synthesized MA-HAP adsorbent were studied to evaluate its suitability for cationic uptake. The incorporated magnetic nanoparticles significantly improved the Co2+ adsorption capacity of MA-HAP to 68.95 mg/g under optimized conditions such as a pH of 6, a contact time of 120 min and an adsorbent dosage of 4 g/L. More than 92% of Co2+ was removed from the simulated aqueous solution in the presence of other ionic-corrosion-products. Densification of the nanocomposite loaded with the corrosion product was carried out using a pressure-assisted cold-sintering technique at 200 °C for 10 min. The sintered waste form showed high relative density (>95%) and hardness (>2.5 GPa). The results of a product consistency test indicated a low normalized leaching rate in the range 10−6 to 10−7 g/m2/day for all ions adsorbed by the MA-HAP. Thus, the material and methods introduced here are highly capable of adsorbing and immobilizing radioactive waste." @default.
- W2900858045 created "2018-11-29" @default.
- W2900858045 creator A5030553175 @default.
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- W2900858045 date "2019-02-01" @default.
- W2900858045 modified "2023-09-27" @default.
- W2900858045 title "Adsorption and immobilization of radioactive ionic-corrosion-products using magnetic hydroxyapatite and cold-sintering for nuclear waste management applications" @default.
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- W2900858045 doi "https://doi.org/10.1016/j.jnucmat.2018.11.026" @default.
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