FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W2914652917> ?p ?o ?g. }

• W2914652917 endingPage "7999" @default.
• W2914652917 startingPage "7990" @default.
• W2914652917 abstract "We studied the kinetics of photoelectrochemical (PEC) water oxidation using a model photoanode BiVO4 modified with various water oxidation catalysts (WOCs) by electrochemical impedance spectroscopy. In particular, we prepared BiVO4 photoanodes with catalytic multilayers (CMs), where cationic polyelectrolytes and anionic polyoxometalate (POM) WOCs were assembled in a desired amount at a nanoscale precision, and compared their performance with those with well-known WOCs such as cobalt phosphate (CoPi) and NiOOH. Our comparative kinetics analysis suggested that the deposition of the CMs improved the kinetics of both the photogenerated charge carrier separation/transport in bulk BiVO4 due to passivation of surface recombination centers and water oxidation at the electrode/electrolyte interface due to deposition of efficient molecular WOCs. On the contrary, the conventional WOCs were mostly effective in the former and less effective in the latter, which is consistent with previous reports. These findings explain why the CMs exhibit an outstanding performance. We also found that separated charge carriers can be efficiently transported to POM WOCs via a hopping mechanism due to the delicate architecture of the CMs, which is reminiscent of natural photosynthetic systems. We believe that this study can not only broaden our understanding on the underlying mechanism of PEC water oxidation but also provide insights for the design and fabrication of novel electrochemical and PEC devices, including efficient water oxidation photoanodes." @default.
• W2914652917 created "2019-02-21" @default.
• W2914652917 creator A5008383067 @default.
• W2914652917 creator A5044053298 @default.
• W2914652917 creator A5072806096 @default.
• W2914652917 creator A5080556920 @default.
• W2914652917 date "2019-02-13" @default.
• W2914652917 modified "2023-10-14" @default.
• W2914652917 title "Catalytic Multilayers for Efficient Solar Water Oxidation through Catalyst Loading and Surface-State Passivation of BiVO₄ Photoanodes" @default.
• W2914652917 cites W1874429410 @default.
• W2914652917 cites W1968076335 @default.
• W2914652917 cites W1983713181 @default.
• W2914652917 cites W1987145056 @default.
• W2914652917 cites W1993194978 @default.
• W2914652917 cites W1993305125 @default.
• W2914652917 cites W1997572663 @default.
• W2914652917 cites W1998243192 @default.
• W2914652917 cites W2008936105 @default.
• W2914652917 cites W2011715705 @default.
• W2914652917 cites W2012752337 @default.
• W2914652917 cites W2044971940 @default.
• W2914652917 cites W2058468006 @default.
• W2914652917 cites W2065174310 @default.
• W2914652917 cites W2070491781 @default.
• W2914652917 cites W2073739962 @default.
• W2914652917 cites W2099469237 @default.
• W2914652917 cites W2104181270 @default.
• W2914652917 cites W2113626928 @default.
• W2914652917 cites W2115607122 @default.
• W2914652917 cites W2137616353 @default.
• W2914652917 cites W2139129883 @default.
• W2914652917 cites W2152769853 @default.
• W2914652917 cites W2158473396 @default.
• W2914652917 cites W2165397960 @default.
• W2914652917 cites W2260329495 @default.
• W2914652917 cites W2324881452 @default.
• W2914652917 cites W2326765563 @default.
• W2914652917 cites W2338926568 @default.
• W2914652917 cites W2460043081 @default.
• W2914652917 cites W2460518522 @default.
• W2914652917 cites W2511079777 @default.
• W2914652917 cites W2569729589 @default.
• W2914652917 cites W2593229437 @default.
• W2914652917 cites W2601760774 @default.
• W2914652917 cites W2606989693 @default.
• W2914652917 cites W2617734483 @default.
• W2914652917 cites W2731790722 @default.
• W2914652917 cites W2765271887 @default.
• W2914652917 cites W2783843627 @default.
• W2914652917 cites W2784407110 @default.
• W2914652917 cites W2791581005 @default.
• W2914652917 cites W2801083710 @default.
• W2914652917 cites W2808346489 @default.
• W2914652917 cites W2810715139 @default.
• W2914652917 cites W2884243765 @default.
• W2914652917 cites W2891316953 @default.
• W2914652917 cites W2894068738 @default.
• W2914652917 cites W2902392934 @default.
• W2914652917 cites W2907621400 @default.
• W2914652917 doi "https://doi.org/10.1021/acsami.8b20785" @default.
• W2914652917 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30757899" @default.
• W2914652917 hasPublicationYear "2019" @default.
• W2914652917 type Work @default.
• W2914652917 sameAs 2914652917 @default.
• W2914652917 citedByCount "28" @default.
• W2914652917 countsByYear W29146529172019 @default.
• W2914652917 countsByYear W29146529172020 @default.
• W2914652917 countsByYear W29146529172021 @default.
• W2914652917 countsByYear W29146529172022 @default.
• W2914652917 countsByYear W29146529172023 @default.
• W2914652917 crossrefType "journal-article" @default.
• W2914652917 hasAuthorship W2914652917A5008383067 @default.
• W2914652917 hasAuthorship W2914652917A5044053298 @default.
• W2914652917 hasAuthorship W2914652917A5072806096 @default.
• W2914652917 hasAuthorship W2914652917A5080556920 @default.
• W2914652917 hasConcept C121332964 @default.
• W2914652917 hasConcept C127413603 @default.
• W2914652917 hasConcept C147789679 @default.
• W2914652917 hasConcept C148898269 @default.
• W2914652917 hasConcept C161790260 @default.
• W2914652917 hasConcept C171250308 @default.
• W2914652917 hasConcept C17525397 @default.
• W2914652917 hasConcept C185592680 @default.
• W2914652917 hasConcept C192562407 @default.
• W2914652917 hasConcept C2777498215 @default.
• W2914652917 hasConcept C2777959998 @default.
• W2914652917 hasConcept C2779227376 @default.
• W2914652917 hasConcept C33574316 @default.
• W2914652917 hasConcept C35590869 @default.
• W2914652917 hasConcept C42360764 @default.
• W2914652917 hasConcept C52859227 @default.
• W2914652917 hasConcept C55493867 @default.
• W2914652917 hasConcept C62520636 @default.
• W2914652917 hasConcept C65165184 @default.
• W2914652917 hasConcept C68801617 @default.
• W2914652917 hasConcept C7040849 @default.
• W2914652917 hasConceptScore W2914652917C121332964 @default.
• W2914652917 hasConceptScore W2914652917C127413603 @default.

• next