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• W2936700684 abstract "Herein, we show the highly enantioselective borylation of unactivated methylene C(sp3)-H bonds in 2-alkylpyridines and 2-alkyl-1,3-azole derivatives using an iridium-BINOL-based chiral monophosphite catalyst system. Quantum chemical calculations using the artificial force induced reaction (AFIR) method suggested that a monophosphite-Ir-tris(boryl) complex generates a narrow chiral reaction pocket where the differentiation of the enantiotopic methylene C-H bonds is accomplished through an assembly of multiple noncovalent interactions." @default.
• W2936700684 created "2019-04-25" @default.
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• W2936700684 date "2019-04-15" @default.
• W2936700684 modified "2023-10-14" @default.
• W2936700684 title "Iridium-Catalyzed Asymmetric Borylation of Unactivated Methylene C(sp³)–H Bonds" @default.
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• W2936700684 doi "https://doi.org/10.1021/jacs.9b01952" @default.
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