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- W2989690307 abstract "A new paradigm to remove toxic chromate anions from aqueous solution by crystallization of chromate-water clusters with imine-linked guanidinium cationic ligands is introduced. The guanidium-based cationic ligand was easily prepared through the imine condensation of an aldehyde and aminoguanidine hydrochloride. The cationic imine-linked guanidinium ligand (BBIG-Cl) showed a high removal capacity (292.5 mg/g) in the solutions. Rapid decontamination of chromate anions from the wastewater by this cationic ligand was resulted from an instantaneous crystallization. The produced guanidium chromate salts have an extremely low solubility (Ksp,BBIG = 8.19 × 10−9). Such superior removal performance of these materials was attributed to the charge-assisted hydrogen bonding between the cationic ligand and chromate-water hydrate anions, which was revealed by the single-crystal X-ray diffraction analysis and density functional theory (DFT) calculations. In addition, the successful recovery of the guanidium-based ligand makes it more attractive for real-world applications." @default.
- W2989690307 created "2019-12-05" @default.
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- W2989690307 date "2020-07-01" @default.
- W2989690307 modified "2023-10-15" @default.
- W2989690307 title "Chromate separation by selective crystallization" @default.
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- W2989690307 doi "https://doi.org/10.1016/j.cclet.2019.11.034" @default.
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