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- W3094885280 abstract "Improving the photo-induced hot charge utilization rate in granular catalysts with specific nanostructure is hindered by limited hot electron production and rapid recombination in plasmonic metal particles; therefore, promoting photo-induced hot charge generation and transfer during the plasmonic process is a vital approach for enhancing plasmonic catalytic performance. In this work, with the intention of constructing Pd-tipped Au nanorod heterostructures to achieve plasmon-enhanced formic acid dehydrogenation, the magnetic-field-derived electromagnetic induction effect is utilized to further boost the generation and transfer of plasmonic hot charges in Au nanorods. By exposing the plasmonic catalytic system to a rotating permanent magnet at 28 °C, formic acid dehydrogenation efficiency was improved by approximately 60%. The improvement rate in the same system can exceed 150% at 45 °C. This enhancement is attributed to the increase in plasmonic hot charges and the suppression of charge recombination based on the electromagnetic induction effect of plasmonic Au nanorods in a rotating magnetic field. This work provides a practical strategy for designing high-activity catalysts regulated via magnetic field for formic acid dehydrogenation." @default.
- W3094885280 created "2020-11-09" @default.
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- W3094885280 date "2021-02-01" @default.
- W3094885280 modified "2023-09-26" @default.
- W3094885280 title "Electromagnetic induction effect induced high-efficiency hot charge generation and transfer in Pd-tipped Au nanorods to boost plasmon-enhanced formic acid dehydrogenation" @default.
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- W3094885280 doi "https://doi.org/10.1016/j.nanoen.2020.105543" @default.
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