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• W3136103056 abstract "Abstract The amino group in the MOF NH 2 ‐MIL‐101(Cr) was post‐synthetically converted into urea‐groups partially using either ethyl isocyanatoacetate, furfuryl isocyanate, p ‐toluenesulfonyl isocyanate or 3‐(triethoxysilyl)propyl isocyanate in acetonitrile. The derived four novel urea‐MOFs exhibit the expected lower BET surface areas and pore volumes than MIL‐101(Cr) and NH 2 ‐MIL‐101(Cr) MOFs but the partially p ‐toluenesulfonyl‐urea‐modified MOF exhibits an outstanding SO 2 adsorption capacity of 823 cm 3 g −1 (corresponding to 36.7 mmol g −1 or 70 wt.% at T=0 °C and 0.9 bar), which is the second highest SO 2 uptake of any known material today – surprisingly even better than for highly porous MIL‐101(Cr) with an uptake of 645 cm 3 g −1 SO 2 under the same conditions. The high uptake is linked to the favorable dipole interactions of SO 2 with the sulfonyl group of the p ‐toluenesulfonyl‐modified MOF." @default.
• W3136103056 created "2021-03-29" @default.
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• W3136103056 date "2021-04-06" @default.
• W3136103056 modified "2023-10-17" @default.
• W3136103056 title "A Series of new Urea‐MOFs Obtained <i>via</i> Post‐synthetic Modification of NH₂‐MIL‐101(Cr): SO₂, CO₂ and H₂O Sorption" @default.
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• W3136103056 doi "https://doi.org/10.1002/zaac.202100023" @default.
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