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- W4205181036 abstract "A 3D nano-aerogel electrocatalyst is produced based on metal Ni combined with Gd2O3 species through a facile hydrogel route. The synthetic method hinges on the fabrication of oxidized carbon nanotubes (OCNTs) crosslinked poly (vinyl alcohol) to form hydrogel, which permits effective catch of highly active Gd2O3/Ni particles after pyrolysis. The designed Gd2O3-Ni heterostructure on carbon nanotubes (Gd2O3-Ni/CNT) is highly efficient for oxygen reduction electrocatalysis. It is found that the half-wave potential (E1/2) of Gd2O3-Ni/CNT is nearly 190 mV positive than that of Ni/CNT and even surpasses the commercial Pt/C. The superior performance is resulted from the electronic reconfiguration between Gd2O3 and Ni in the heterostructure, which further optimized the adsorption of intermediates to balance the binding of OOH* and OH* on the surface of Gd2O3-Ni and break the OOH*–OH* scaling relation. Finally, the assembled zinc-air battery with Gd2O3-Ni/CNT as electrocatalyst achieves high capacity." @default.
- W4205181036 created "2022-01-25" @default.
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- W4205181036 date "2022-04-01" @default.
- W4205181036 modified "2023-09-27" @default.
- W4205181036 title "Engineering Gd2O3-Ni heterostructure for efficient oxygen reduction electrocatalysis via the electronic reconfiguration and adsorption optimization of intermediates" @default.
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- W4205181036 doi "https://doi.org/10.1016/j.cej.2022.134597" @default.
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