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• W4302007611 abstract "Famous as emerging inorganic-organic hybrid materials, metal-organic frameworks (MOFs) and MOF-based composites have been displaying bright prospects in catalysis fields. It is desirable to develop highly efficient MOF-based catalysts with excellent activity, selectivity, and stability. The nanostructure of MOFs can bring dramatic effects on their inherent physical/chemical properties and the interaction with reaction substrates/intermediates. Therefore, it is applicable to promote the performance of MOF-based catalysts via nanostructure engineering. In this review, we focus on four classes of nanostructures, i.e., ultrathin nanostructure, hierarchically porous nanostructure, defective nanostructure, and MOF-shelled nanostructure (composite with MOF shell). Strategies for nanostructure engineering of MOF-based catalysts are summarized, their applications in thermo-catalysis, electrocatalysis, and photocatalysis are overviewed, and the effects of nanostructure engineering on catalytic performance are discussed. We hope this review will be instructive for researchers in the rational and controllable construction of MOF nanostructures for catalytic performance promotions. Famous as emerging inorganic-organic hybrid materials, metal-organic frameworks (MOFs) and MOF-based composites have been displaying bright prospects in catalysis fields. It is desirable to develop highly efficient MOF-based catalysts with excellent activity, selectivity, and stability. The nanostructure of MOFs can bring dramatic effects on their inherent physical/chemical properties and the interaction with reaction substrates/intermediates. Therefore, it is applicable to promote the performance of MOF-based catalysts via nanostructure engineering. In this review, we focus on four classes of nanostructures, i.e., ultrathin nanostructure, hierarchically porous nanostructure, defective nanostructure, and MOF-shelled nanostructure (composite with MOF shell). Strategies for nanostructure engineering of MOF-based catalysts are summarized, their applications in thermo-catalysis, electrocatalysis, and photocatalysis are overviewed, and the effects of nanostructure engineering on catalytic performance are discussed. We hope this review will be instructive for researchers in the rational and controllable construction of MOF nanostructures for catalytic performance promotions." @default.
• W4302007611 created "2022-10-06" @default.
• W4302007611 creator A5008668835 @default.
• W4302007611 creator A5009643462 @default.
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• W4302007611 creator A5053555867 @default.
• W4302007611 creator A5070596342 @default.
• W4302007611 creator A5085096969 @default.
• W4302007611 date "2022-10-01" @default.
• W4302007611 modified "2023-10-15" @default.
• W4302007611 title "Nanostructural engineering of metal-organic frameworks: Construction strategies and catalytic applications" @default.
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